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OH and O radicals production in atmospheric pressure air/Ar/H_2O gliding arc discharge plasma jet

OH and O radicals production in atmospheric pressure air/Ar/H_2O gliding arc discharge plasma jet

作     者:N C ROY M R TALUKDER A N CHOWDHURY 

作者机构:Plasma Science and Technology LaboratoryDepartment of Applied Physics and Electronic EngineeringUniversity of RajshahiRajshahi 6205Bangladesh Bangladesh Council of Scientific and Industrial Research Laboratory RajshahiRajshahi 6206Bangladesh 

出 版 物:《Plasma Science and Technology》 (等离子体科学和技术(英文版))

年 卷 期:2017年第19卷第12期

页      面:71-80页

核心收录:

学科分类:07[理学] 070204[理学-等离子体物理] 0702[理学-物理学] 

基  金:financial support has been provided by the University Grants Commission:A-663-5/52/UGC/Eng-9/2013 and A-670-5/52/UGC/Eng-4/2013 University of Rajshahi 

主  题:reactive oxygen species(ROS) optical emission spectroscopy(OES) gliding arc discharge plasma kinetics broadening mechanism 

摘      要:Atmospheric pressure air/Ar/H_2O gliding arc discharge plasma is produced by a pulsed dc power supply. An optical emission spectroscopic(OES) diagnostic technique is used for the characterization of plasmas and for identifications of OH and O radicals along with other species in the plasmas. The OES diagnostic technique reveals the excitation Tx?≈?5550–9000 K, rotational Tr?≈?1350–2700 K and gas Tg?≈?850–1600 K temperatures, and electron density n?(1.1-1.9) ′101 4 cm^(-3) e under different experimental conditions. The production and destruction of OH and O radicals are investigated as functions of applied voltage and air flow rate. Relative intensities of OH and O radicals indicate that their production rates are increased with increasing Ar content in the gas mixture and applied voltage. nereveals that the higher densities of OH and O radicals are produced in the discharge due to more effective electron impact dissociation of H_2O and O_2 molecules caused by higher kinetic energies as gained by electrons from the enhanced electric field as well as by enhanced n *** productions of OH and O are decreasing with increasing air flow rate due to removal of Joule heat from the discharge region but enhanced air flow rate significantly modifies discharge maintenance properties. Besides, Tgsignificantly reduces with the enhanced air flow rate. This investigation reveals that Ar plays a significant role in the production of OH and O radicals.

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