Advances in direct production of value-added chemicals via syngas conversion

作     者：Yunlei An Tiejun Lin Fei Yu Yanzhang Yang Liangshu Zhong Minghong Wu Yuhan Sun 

作者机构：School of Environmental and Chemical EngineeringShanghai UniversityShanghai 200444China CAS Key Laboratory of Low-Carbon Conversion Science and EngineeringShanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201203China University of the Chinese Academy of SciencesBeijing 100049China School of Physical Science and TechnologyShanghaiTech UniversityShanghai 201203China 

出 版 物：《Science China Chemistry》 (中国科学（化学英文版）)

年 卷 期：2017年第60卷第7期

页      面：887-903页

核心收录：

学科分类：0817[工学-化学工程与技术] 08[工学] 

基　　金：supported by the National Natural Science Foundation of China(91545112,21573271,21403278) Shanghai Municipal Science and Technology Commission,China(15DZ1170500) the Chinese Academy of Sciences(QYZDB-SSW-SLH035) 

主　　题：green carbon science syngas conversion Fischer Tropsh Fischer Tropsh to olefins higher alcohol synthesis 

摘      要：Syngas conversion to fuels and chemicals is one of the most challenging subjects in the field of C1 chemistry. It is considered as an attractive alternative non-petroleum-based production route. The direct synthesis of olefins and alcohols as high value-added chemicals from syngas has drawn particular attention due to its process simplicity, low energy consumption and clean utilization of carbon resource, which conforms to the principles of green carbon science. This review describes the recent advances for the direct production of lower olefins and higher alcohols via syngas conversion. Recent progress in the development of new catalyst systems for enhanced catalytic performance is highlighted. We also give recommendations regarding major challenges for further research in syngas conversion to various chemicals.