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Vapor transport growth of MoS2 nucleated on SiO2 patterns and graphene flakes

Vapor transport growth of MoS2 nucleated on SiO2 patterns and graphene flakes

作     者:Toma Stoica Mihai Stoica Martial Duchamp Andreas Tiedemann Siegfried Mantl Detlev Orutzmacher Dan Buca Beata E. Kardynal 

作者机构:Peter Grunberg Institute 9 (PGI 9) andJARA-Fundamentals of Future Information Technologies Forschungszentrum Julich Julich 52425 Germany National Institute of Materials Physics Magurele Bucharest 077125 Romania Institute of Physical Chemistry 'llie Murgulescu' of the Romanian Academy Bucharest 060021 Romania Peter Grunberg Institute 5 (PGI 5) and JARA-Fundamentals of Future Information Technologies Forschungszentrum Julich Julich 52425 Germany 

出 版 物:《Nano Research》 (纳米研究(英文版))

年 卷 期:2016年第9卷第11期

页      面:3504-3514页

核心收录:

学科分类:07[理学] 

基  金:support from Helmholtz-DAAD Fellowship NIMP Core Program project 

主  题:MoS2 localized nucleation andgrowth graphene two-dimensional (2D)heterostructures 

摘      要:Vapor transport growth of atomically thin MoS2 layers on patterned substrates is investigated, as it is a step towards the self-aligned growth and formation of heterojunctions, which could be useful in future applications. Enhanced formation of MoS2 flakes at the pattern edges is observed on both the substrates examined, namely, patterned thermal SiO2 on Si(100) and graphene flakes on SiO2. The diffusion driven growth leads to the formation of MoS2 monolayers (MLs) with sizes of tens of micrometers around the edges of SiO2 patterns. The growth mode and the optical quality of the MoS2 flakes can be controlled by varying the substrate temperature. Besides the lateral growth, 3R-type pyramids are obtained on prolonging the growth. Lateral MoS2-graphene heterostructures are obtained by using graphene flakes on SiO2 as a substrate.

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