Heterojunction between anodic TiO_2/g-C_3N_4 and cathodic WO_3/W nano-catalysts for coupled pollutant removal in a self-biased system
阳极TiO_2/g-C_3N_4与阴极WO_3/W纳米催化剂之间扩大的异质结自偏压系统去除污染物(英文)作者机构:大连理工大学环境学院工业生态与环境工程教育部重点实验室辽宁大连116024 大连理工大学食品与环境学院辽宁盘锦124221
出 版 物:《Chinese Journal of Catalysis》 (催化学报(英文))
年 卷 期:2017年第38卷第2期
页 面:270-277页
核心收录:
学科分类:083002[工学-环境工程] 0830[工学-环境科学与工程(可授工学、理学、农学学位)] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术]
基 金:supported by the National Natural Science Foundation of China (21177018, 21677025) the Program of Introducing Talents of Discipline to Universities (B13012)
主 题:Self-biased system Hetero-junction No light irradiation Low energy consumption Pollutant degradation
摘 要:An anodic TiO2/g-C3N4 hetero-junction and cathodic WO3/W were used to build a self-sustained catalytic fuel cell system for oxidizing rhodamine B or triclosan and reducing NO3^--N to N2 *** WO3 nano-catalyst was formed in situ by heating and oxidizing a tungsten wire in *** voltammetry and current-time curves were used to characterize the electrochemical properties of the electrodes and *** and activation of molecular oxygen by self-biased TiO2/g-C3N4 led to the formation of reactive oxidizing species in the fuel *** mechanism of simultaneous anodic oxidation of pollutants and cathodic reduction of nitrate was *** spontaneously formed circuit and tiny current were used simultaneously in treating two kinds of wastewater in the reactor chambers,even without light illumination or an external applied *** new catalytic pollution control route can lower energy consumption and degrade many other kinds of pollutants.