Electrocatalytic coupling of anodic nitrogen oxidation and cathodic nitrate reduction for ammonia synthesis from air and water
作者机构：State Key Laboratory of Separation Membranes and Membrane ProcessesTianjin Key Laboratory of Green Chemical Technology and Process EngineeringSchool of Chemical Engineering and TechnologyTiangong UniversityTianjin 300387China Institute of Molecular PlusSchool of Chemical EngineeringTianjin UniversityTianjin 300072China
出 版 物：《Nano Research》 (纳米研究（英文版）)
年 卷 期：2024年第17卷第9期
页 面：7824-7829页
核心收录：
学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070303[理学-有机化学] 0703[理学-化学]
基 金：supported by Tianjin Science and Technology Program(No.22ZYJDSS00060) Program for Tianjin Innovative Research Team in Universities(No.TD13-5031) Tianjin 131 Research Team of Innovative Talents the National Natural Science Foundation of China(No.22109115) the Special Fund for Postgraduate Education(No.B1-2021-010)for financial support
主 题：electrocatalysis nitrogen oxidation nitrate reduction nitrogen fixation ammonia synthesis
摘 要：Ammonia plays a vital role in present agriculture and industry,and is also regarded as a next-generation clean energy *** development of electrocatalysis raises an opportunity to make ammonia synthesis compatible with intermittent and variable renewable energy sources such as solar and wind ***,the direct ammonia electrosynthesis from N_(2)reduction is still challenging due to the much easier hydrogen evolution competition *** this perspective,we propose a novel strategy for ammonia electrosynthesis from air and water based on the coupling of anodic nitrogen oxidation and cathodic nitrate *** methods for breaking the bottlenecks of anodic nitrogen oxidation and cathodic nitrate reduction are discussed *** that,key issues that need to be considered in the coupled system are proposed for the application of this strategy.
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