Halide perovskite-based heterostructures for photocatalytic CO_(2)conversion

作     者：Yue-Mei Li Zhuang-Zhuang Hou Xiao-Dong Wan Jia Liu Jia-Tao Zhang 

作者机构：School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Institute of Radio MeasurementBeijing 100854China School of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China 

出 版 物：《Rare Metals》 (稀有金属（英文版）)

年 卷 期：2024年第43卷第11期

页      面：5453-5472页

核心收录：

学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070303[理学-有机化学] 0703[理学-化学] 

基　　金：financially supported by the National Natural Science Foundation of China(Nos.52072035 and 52272186) 

主　　题：Halide perovskite Heterostructures Photocatalysis CO_(2)reduction 

摘      要：Photocatalytic conversion of solar light into chemical fuels represents an appealing pathway by which a sustainable energy future might be ***,great scientific challenges need to be addressed for developing this technology,such as finding a way to acquire highly efficient semiconductor photocatalytic ***,halide perovskites have emerged as a novel class of semiconductors that display several exceptional advantages,including a large absorption coefficient,high carrier mobility,as well as customizable tunability of band gap,composition,structures,and *** development of photocatalysts solely based on pure halide perovskites encounters significant hurdles due to their intrinsically low stability and activity.A promising strategy to overcome this problem involves the construction of perovskite-based *** integration with other components can enhance light absorption capacity,promote the separation of photogenerated carriers,and augment the number of surface reactive *** this review,we briefly summarize recent advances in the construction of perovskite-based photocatalytic heterostructures,where the perovskites serve either as the matrix or as a decoration ***,the research accomplishments in employing these heterostructures for photocatalytic CO_(2)reduction are ***,the major obstacles and the great potential for future design of perovskite-based heterostructures toward the creation of competitive CO_(2)conversion photocatalysts are proposed.