Metal−support interaction in single-atom electrocatalysts:A perspective of metal oxide supports
作者机构：State Key Laboratory of Electroanalytical ChemistryJilin Province Key Laboratory of Low Carbon Chemical PowerChangchun Institute of Applied ChemistryChinese Academy of Sciences5625 Renmin StreetChangchunJilin 130022China School of Applied Chemistry and EngineeringUniversity of Science and Technology of ChinaHefeiAnhui 230026China
出 版 物：《eScience》 (电化学与能源科学（英文）)
年 卷 期：2024年第4卷第5期
页 面：1-9页
学科分类：081704[工学-应用化学] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0703[理学-化学]
基 金：The authors are grateful to the financial support from the Key Research and Development Program sponsored by the Ministry of Science and Technology(MOST)(2022YFA1203400) the National Natural Science Foundation of China(22102172,22372155,22072145,22005294,21925205,21721003) the authors also thank the ZEROVISION company for providing assistance in creating figures for this manuscript
主 题：Single-atom catalyst Metal oxide Electrocatalysis Metal-support interaction
摘 要：The discovery of single-atom catalysts(SACs)represents a groundbreaking advancement in the field of catalysis over the past *** the in-depth exploration of relevant structure-activity relationships,the metal−support interaction(MSI)is widely adopted to elucidate variations in electronic structure and coordination configuration of atomic active sites on various kinds of ***,we briefly summarize the metal oxide supports for SACs fabrication,including the distinctive characteristics of metal oxide supports,enlightening advancements in metal oxide support-based SACs(MO-SACs),feasible preparation methods for MO-SACs and effective regulation strategies of MSI effect in *** addition,we present our viewpoints and outlook in this field to stimulate rational design and construction of novel MO-SACs applied in diverse renewable energy devices,while some universal suggestions are sincerely given to provoke thoughtful considerations during the research process.
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