Ethanol-assisted synthesis of a Ni single-atom catalyst with poriferous 3D framework for efficient cascade CO_(2)electroreduction

作     者：Feng Wu Shi-Qi Wang Sebastian Kunze Xiao-Ping Gao Pei-Qun Yin Yu-En Wu Feng Wu;Shi-Qi Wang;Sebastian Kunze;Xiao-Ping Gao;Pei-Qun Yin;Yu-En Wu

作者机构：Division of Life Sciences and MedicineDepartment of EndocrinologySchool of Chemistry and Materials ScienceThe First Affiliated Hospital of USTCUniversity of Science and Technology of ChinaHefei 230026China Department of ChemistrySeoul National UniversitySeoul 08826South Korea School of Biomedical EngineeringAnhui Medical UniversityHefei 230032China 

出 版 物：《Rare Metals》 (稀有金属（英文版）)

年 卷 期：2024年第43卷第9期

页      面：4612-4619页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 

基　　金：supported by China Ministry of Science and Technology(No.2020YFA0710203) the Collaborative Innovation Program of Hefei Science Center,CAS(No.2021HSC-CIP002) the Joint Funds from Hefei National Synchrotron Radiation Laboratory(No.KY2060000195) 

主　　题：reaction. synthesis catalyst 

摘      要：The electroreduction of carbon dioxide to generate multicarbon products is significant for achieving a carbon-neutral ***,the selectivity for multi-carbon products faces several challenges,such as the intricate nature of the multistep hydrogenation processes,slow reaction kinetics and the bicarbonate precipitate issue caused by alkaline *** factors hinder the extensive utilization of this ***,we successfully developed and implemented a tandem electrolyzer cascade to separate and optimize the complex elementary reactions involved in the process of multi-carbon production.