Two-dimensional semiconductor heterostructures for photocatalytic CO_(2)conversion

作     者：Yang Wu Mingyu Wu Yongfu Sun Yi Xie 

作者机构：Hefei National Research Center for Physical Sciences at MicroscaleUniversity of Science and Technology of ChinaHefei 230026China 

出 版 物：《Science China Chemistry》 (中国科学（化学英文版）)

年 卷 期：2024年第67卷第8期

页      面：2434-2447页

核心收录：

学科分类：081704[工学-应用化学] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0703[理学-化学] 

基　　金：financially supported by the National Key R&D Program of China(2019YFA0210004,2022YFA1502904,2022YFA1203600) National Natural Science Foundation of China(22125503,52394201,22321001,U2032212) 

主　　题：two-dimensional semiconductor heterostructures photocatalysis CO_(2)conversion 

摘      要：The CO_(2)reduction into carbon-contained fuel via solar energy offers the powerful tools to realize the zero-emission carbon *** to the intriguing features of the two-dimensional(2D)heterostructures,it is susceptible to modulate the electronic structure as well as the surface geometry for optimizing the photocatalytic CO_(2)*** this perspective,we surveyed the fundamental insights of 2D semiconductor heterostructures,involving the fabrication strategies and classification of the 2D semiconductor ***,we have detailly discussed the overview of 2D semiconductor heterostructure for optimizing CO_(2)photocatalytic influenced factors,including the solar energy utilization,photogenerated carriers separation,and redox reaction ***,we showed the significant advantages of 2D heterostructures in elevating CO_(2)photoreduction performance,focusing on activity,selectivity and *** analyzing the limitations and developments,we ended by putting forward insights into the further researches about the CO_(2)photocatalysts and reactor design,even industrial applications.