Recent progress on the synthesis of defective UiO-66 for thermal catalysis

作     者：Qing Feng Caoyu Yang Lin Chang Guodong Li Zhiyong Tang 

作者机构：CAS Key Laboratory of Nanosystem and Hierarchical FabricationCAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China School of Nanoscience and EngineeringUniversity of Chinese Academy of SciencesBeijing 100049China 

出 版 物：《Nano Research》 (纳米研究（英文版）)

年 卷 期：2024年第17卷第10期

页      面：8653-8670页

核心收录：

学科分类：081704[工学-应用化学] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0703[理学-化学] 

基　　金：the National Key Research and Development Program of China(No.2021YFA1500403,G.D.L.,Nos.2021YFA1200302 and 2022YFA1205400,Z.Y.T.) Strategic Priority Research Program of Chinese Academy of Sciences(No.XDB36000000,Z.Y.T.and G.D.L.) National Natural Science Foundation of China(Nos.92356304 and 92056204,Z.Y.T.,Nos.52372079 and 22173024,G.D.L.,No.52003066,L.C.) Youth Innovation Promotion Association of CAS(G.D.L.) 

主　　题：defective UiO-66 de novo synthesis post-synthetic treatment characterization thermal catalysis 

摘      要：Zirconium terephthalate UiO-66 has aroused great interest in catalysis since it exhibits significant flexibility and compatibility for accommodating a high number of defects as well as exceptional thermal and chemical *** now,many works have focused on the modulations of the Zr6-oxo clusters in UiO-66 in terms of diverse synthesis,advanced characterizations,and their catalytic *** achieve high catalytic efficiency,it is still highly desired for rationally constructing and modulating the Zr6-oxo clusters with exposed catalytic sites and diverse microenvironments for advanced *** this review,we provide a comprehensive summary of recent progress on the synthesis of defective UiO-66,qualitative and quantitative characterizations,as well as a logical overview of heterogeneous catalytic applications over the past few ***,the outlooks for the research paradigm of defective UiO-66 are discussed.