Recent advances and perspectives in MXene-based cathodes for aqueous zinc-ion batteries

作     者：Aiduo Wu Tianhao Wang Long Zhang Chen Chen Qiaomin Li Xuanhui Qu Yongchang Liu Aiduo Wu;Tianhao Wang;Long Zhang;Chen Chen;Qiaomin Li;Xuanhui Qu;Yongchang Liu

作者机构：Beijing Advanced Innovation Center for Materials Genome EngineeringInstitute for Advanced Materials and TechnologyState Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing 100083China School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China School of Economics and ManagementUniversity of Science and Technology BeijingBeijing 100083China 

出 版 物：《International Journal of Minerals,Metallurgy and Materials》 (矿物冶金与材料学报（英文版）)

年 卷 期：2024年第31卷第7期

页      面：1752-1765页

核心收录：

学科分类：0819[工学-矿业工程] 0808[工学-电气工程] 0806[工学-冶金工程] 08[工学] 080501[工学-材料物理与化学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：the National Natural Science Foundation of China(Nos.52372171,22075016,and 52201201) the National Program for Support of Top-notch Young Professionals,China the Interdisciplinary Research Project for Young Teachers of University of Science and Technology Beijing,China(No.FRF-IDRY-21-011) the State Key Laboratory for Advanced Metals and Materials,China(No.2022Z-17) the Ministry of Education Social Science Project,China(No.18YJC790087) the“Xiaomi Young Scholar”Funding Project,China,and the 111 Project,China(No.B170003) 

主　　题：aqueous zinc-ion batteries MXenes terminal groups interlayer engineering conductive network design 

摘      要：Aqueous zinc-ion batteries(AZIBs)show great potential for applications in grid-scale energy storage,given their intrinsic safety,cost effectiveness,environmental friendliness,and impressive electrochemical ***,strong electrostatic interactions exist between zinc ions and host materials,and they hinder the development of advanced cathode materials for efficient,rapid,and stable Zn-ion *** and their derivatives possess a large interlayer spacing,excellent hydrophilicity,outstanding electronic conductivity,and high redox *** materials are considered“rising starcathode candidates for *** comprehensive review discusses recent advances in MXenes as AZIB cathodes from the perspectives of crystal structure,Zn-storage mechanism,surface modification,interlayer engineering,and conductive network design to elucidate the correlations among their composition,structure,and electrochemical *** work also outlines the remaining challenges faced by MXenes for aqueous Zn-ion storage,such as the urgent need for improved toxic preparation methods,exploration of potential novel MXene cathodes,and suppression of layered MXene restacking upon cycling,and introduces the prospects of MXene-based cathode materials for high-performance AZIBs.