Effect of gas components on the postdischarge temporal behavior of OH and O of a non-equilibrium atmospheric pressure plasma driven by nanosecond voltage pulses

作     者：王兰萍 聂兰兰 卢新培 Lanping WANG;Lanlan NIE;Xinpei LU

作者机构：State Key Laboratory of Advanced Electromagnetic Engineering and TechnologySchool of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China 

出 版 物：《Plasma Science and Technology》 (等离子体科学和技术（英文版）)

年 卷 期：2024年第26卷第5期

页      面：72-81页

核心收录：

学科分类：07[理学] 070204[理学-等离子体物理] 0702[理学-物理学] 

基　　金：supported by National Natural Science Foundation of China(Nos.52130701 and 51977096) the National Key Research and Development Program of China(No.2021YFE0114700) 

主　　题：O atom OH radical post-discharge temporal behavior laser-induced fluorescence 

摘      要：OH radicals and O atoms are two of the most important reactive species of non-equilibrium atmospheric pressure plasma(NAPP),which plays an important role in applications such as plasma ***,experimental studies on how the gas content affects the postdischarge temporal evolutions of OH and O in the noble gas ns-NAPP are very *** this work,the effect of the percentages of O_(2),N_(2),and H_(2)O on the amounts of OH and O productions and their post-discharge temporal behaviors in ns-NAPP is investigated by laser-induced fluorescence(LIF)*** results show that the productions of OH and O increase and then decrease with the increase of O_(2)*** OH and O densities reach their maximum when about 0.8%O_(2)is *** increase of the O_(2)concentration results in a decrease of the initial densities of both OH and O,and leads to their faster *** increase of N_(2)percentage also results in the increase and then decrease of the OH and O densities,but the change is ***,when the H_(2)O concentration is increased from 100 to 3000 ppm,the initial OH density increases slightly,but the OH density decays much faster,while the initial density of O decreases with the increase of the H_(2)O *** analysis,it is found that OH and O are mainly produced through electron collisional dissociation.O(^(1)D)is critical for OH generation.O_(3)accelerates the consumption processes of OH and O at high O_(2)*** addition of H_(2)O in the NAPP considerably enhances the electronegativity,while it decreases the overall plasma reactivity,accelerates the decay of OH,and reduces the O atom density.