Defect engineering in transition-metal(Fe,Co,andNi)-based electrocatalysts for water splitting

作     者：Kaili Wu Chaojie Lyu Jiarun Cheng Weifan Ding Jiwen Wu Qian Wang Woon-Ming Lau Jinlong Zheng 

作者机构：Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijingChina School of Chemistry and Chemical EngineeringLinyi UniversityLinyiChina Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijingChina Shunde Innovation SchoolUniversity of Science and Technology BeijingFoshanChina 

出 版 物：《Carbon Energy》 (碳能源（英文）)

年 卷 期：2024年第6卷第6期

页      面：165-199页

核心收录：

学科分类：081704[工学-应用化学] 08[工学] 0817[工学-化学工程与技术] 

基　　金：National Natural Science Foundation of China,Grant/Award Number:52271200 Scientific and Technological Innovation Foundation of Foshan,Grant/Award Number:BK20BE009 the Fundamental Research Funds for the Central Universities,Grant/Award Number:FRF-TP-18-079A1 Guangdong Basic and Applied Basic Research Foundation,Grant/Award Number:2020A1515110460,ORCID:http://orcid.org/0000-0002-0870-2248 

主　　题：defect engineering electrocatalytic water splitting element doping interfacial engineering vacancy 

摘      要：Electrocatalytic water splitting seems to be an efficient strategy to deal with increasingly serious environmental problems and energy crises but still suffers from the lack of stable and efficient *** practical electrocatalysts by introducing defect engineering,such as hybrid structure,surface vacancies,functional modification,and structural distortions,is proven to be a dependable solution for fabricating electrocatalysts with high catalytic activities,robust stability,and good *** review is an overview of some relevant reports about the effects of defect engineering on the electrocatalytic water splitting performance of *** detail,the types of defects,the preparation and characterization methods,and catalytic performances of electrocatalysts are presented,emphasizing the effects of the introduced defects on the electronic structures of electrocatalysts and the optimization of the intermediates adsorption energy throughout the ***,the existing challenges and personal perspectives of possible strategies for enhancing the catalytic performances of electrocatalysts are *** in-depth understanding of the effects of defect engineering on the catalytic performance of electrocatalysts will light the way to design high-efficiency electrocatalysts for water splitting and other possible applications.