Challenges in Photocatalytic Carbon Dioxide Reduction
作者机构：National Forestry and Grassland Administration Key Laboratory of Plant Fiber Functional MaterialsCollege of Material EngineeringFujian Agriculture and Forestry UniversityFuzhou 350002China School of Chemistry and Chemical Engineering/State Key Laboratory Incubation Base for Green Processing of Chemical EngineeringShihezi UniversityShihezi 832003China College of Ecological Environment and Urban ConstructionFujian University of TechnologyFuzhou 350118China
出 版 物：《Precision Chemistry》 (精准化学（英文）)
年 卷 期：2024年第2卷第2期
页 面：49-56页
学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070303[理学-有机化学] 0703[理学-化学]
基 金：This work was supported by the National Natural Science Foundation of China(Grant No.52203110) the Natural Science Foundation of Fujian Province(Grant No.2023J05052) the Knowledge Innovation Program of Wuhan-Shuguang Project(Grant No.2022010801020216) the School of Chemistry and Chemical Engineering/State Key Laboratory Incubation Base for Green Processing of Chemical Engineering,Shihezi,832003,China
主 题：Phtocatalytic CO_(2)reduction Reaction Pathways Product Selectivity Charge Transfer Mechanism Overestimate of Product Yield
摘 要：An energy crisis and significant anthropogenic CO_(2)emissions as a result of rising fossil fuel consumption have caused a rapid increase in global *** of the best solutions to these two issues is thought to be the photocatalytic reduction of CO_(2)into value-added carbon-containing *** this aspect,the main challenges mainly include the photocatalytic mechanism,reaction activity,and product selectivity,especially in ambiguous reaction pathways and product selectivity,an unclear charge transfer mechanism,and an overestimate of product ***,in this perspective,we attempt to exhibit the discussion and in-depth analysis of the possible reaction pathways and product selectivity,the specific charge transfer mechanism,and the origin of carbon-containing products in phtocatalytic CO_(2)***,the fundamentals for photocatalytic CO_(2)reduction are also ***,the state-of-the-art challenges and perspectives in CO_(2)photoreduction are highlighted and discussed in *** perspective is expected to evoke more research attention for the photocatalytic reduction of CO_(2)into value-added products.
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