Deformable Catalytic Material Derived from Mechanical Flexibility for Hydrogen Evolution Reaction

作     者：Fengshun Wang Lingbin Xie Ning Sun Ting Zhi Mengyang Zhang Yang Liu Zhongzhong Luo Lanhua Yi Qiang Zhao Longlu Wang Fengshun Wang;Lingbin Xie;Ning Sun;Ting Zhi;Mengyang Zhang;Yang Liu;Zhongzhong Luo;Lanhua Yi;Qiang Zhao;Longlu Wang

作者机构：College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology)Nanjing University of Posts&Telecommunications(NJUPT)9 WenyuanNanjing 210023People’s Republic of China Key Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of EducationSchool of ChemistryXiangtan UniversityXiangtan 411105People’s Republic of China State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for BiosensorsInstitute of Advanced Materials(IAM)&Institute of Flexible Electronics(Future Technology)Nanjing University of Posts&Telecommunications9 WenyuanNanjing 210023People’s Republic of China 

出 版 物：《Nano-Micro Letters》 (纳微快报（英文版）)

年 卷 期：2024年第16卷第2期

页      面：287-311页

核心收录：

学科分类：081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 0805[工学-材料科学与工程（可授工学、理学学位）] 0702[理学-物理学] 

基　　金：This work was financially supported by the National Natural Science Foundation of China(Nos.51902101 and 21875203) the Natural Science Foundation of Hunan Province(Nos.2021JJ40044 and 2023JJ50287) Natural Science Foundation of Jiangsu Province(No.BK20201381). 

主　　题：Deformable catalytic material Micro-nanostructures evolution Mechanical flexibility Hydrogen evolution reaction 

摘      要：Deformable catalytic material with excellent flexible structure is a new type of catalyst that has been applied in various chemical reactions,especially electrocatalytic hydrogen evolution reaction(HER).In recent years,deformable catalysts for HER have made great progress and would become a research hotspot.The catalytic activities of deformable catalysts could be adjustable by the strain engineering and surface reconfiguration.The surface curvature of flexible catalytic materials is closely related to the electrocatalytic HER properties.Here,firstly,we systematically summarized self-adaptive catalytic performance of deformable catalysts and various micro–nanostructures evolution in catalytic HER process.Secondly,a series of strategies to design highly active catalysts based on the mechanical flexibility of lowdimensional nanomaterials were summarized.Last but not least,we presented the challenges and prospects of the study of flexible and deformable micro–nanostructures of electrocatalysts,which would further deepen the understanding of catalytic mechanisms of deformable HER catalyst.