In-situ template etching synthesis of BiON/BiOCl_(0.9)I_(0.1) heterojunction for photocatalytic degradation of tetracycline
作者机构:School of Chemistry and Chemical EngineeringUniversity of JinanJinan 250022China
出 版 物:《ChemPhysMater》 (化学物理材料(英文))
年 卷 期:2024年第3卷第1期
页 面:103-110页
学科分类:081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术]
基 金:supported by the National Natural Science Foun-dation of China(Grant Nos.52001136,52171179) the project funded by the China Postdoctoral Science Foundation(2020M671981,2021T140269)
主 题:Heterojunction Tetracycline reduction Visible light Photocatalysis
摘 要:Hierarchical heterostructures have emerged as promising candidates for the efficient photocatalytic degradation of antibiotics owing to their matched energy levels and tunable absorption ***,we report the facile synthesis of a heterojunction photocatalyst composed of basic bismuth nitrate(BiON)and BiOCl_(0.9)I_(0.1) using a simple room-temperature hydrolysis *** results demonstrate that the BiON/BiOCl_(0.9)I_(0.1) composite exhibits superior photodegradation performance compared to pure-phase materials owing to the catalytic enhancement at the heterointerface and the effective separation of the photogenerated ***,the unique three-dimensional microsphere morphology of the synthesized composite enhances its specific surface area and light absorption,further enhancing its photocatalytic *** the tetracycline(TC)photodegradation reaction as a model reaction,the catalyst could degrade 88%of TC in just 25 ***,this work provides a promising strategy for the facile and low-cost synthesis of heterogeneous photocatalytic degradation materials.