Designing metal sulfide-based cathodes and separators for suppressing polysulfide shuttling in lithium-sulfur batteries
作者机构:Institute of Advanced Materials and Flexible Electronics(IAMFE)School of Chemistry and Materials ScienceNanjing University of Information Science&TechnologyNanjing 210044China School of Materials Science and EngineeringAnhui University of TechnologyMaanshan 243002China School of Mechanical EngineeringJiangsu University of TechnologyChangzhou 213001China
出 版 物:《Nano Research》 (纳米研究(英文版))
年 卷 期:2024年第17卷第4期
页 面:2574-2591页
核心收录:
学科分类:0808[工学-电气工程] 08[工学] 0805[工学-材料科学与工程(可授工学、理学学位)] 0703[理学-化学] 0702[理学-物理学]
基 金:supported by the open research fund of the State Key Laboratory of Organic Electronics and Information Displays,the Startup Foundation for Introducing Talent of NUIST(Nos.2021r090 and 2021r091) Jiangsu Provincial Scientific Research and Practice Innovation Program(Nos.SJCX23_0420 and SJCX23_0421)
主 题:lithium-sulfur batteries metal sulfides polysulfide shuttling sulfur hosts separator coating layers
摘 要:Lithium-sulfur(Li-S)batteries,known for their high energy density,are attracting extensive research interest as a promising next-generation energy storage ***,their widespread use has been hampered by certain issues,including the dissolution and migration of polysulfides,along with sluggish redox *** sulfides present a promising solution to these obstacles regarding their high electrical conductivity,strong chemical adsorption with polysulfides,and remarkable electrocatalytic capabilities for polysulfide *** this review,the recent progress on the utilization of metal sulfide for suppressing polysulfide shuttling in Li-S batteries is systematically summarized,with a special focus on sulfur hosts and functional *** critical roles of metal sulfides in realizing high-performing Li-S batteries have been comprehensively discussed by correlating the materials’structure and electrochemical ***,the remaining issues/challenges and future perspectives are *** offering a detailed understanding of the crucial roles of metal sulfides,this review dedicates to contributing valuable knowledge for the pursuit of high-efficiency Li-S batteries based on metal sulfides.