Design strategies for rechargeable aqueous metal-ion batteries

作     者：Yang Li Xin Zhao Yifu Gao Yichen Ding Zhichun Si Liubing Dong Dong Zhou Feiyu Kang 

作者机构：Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China College of Chemistry and Materials ScienceJinan UniversityGuangzhou 511443China 

出 版 物：《Science China Chemistry》 (中国科学（化学英文版）)

年 卷 期：2024年第67卷第1期

页      面：165-190页

核心收录：

学科分类：0808[工学-电气工程] 08[工学] 0703[理学-化学] 

基　　金：supported by National Key Research and Development Program of China(2022YFB2404500) Shenzhen Outstanding Talents Training Fund 

主　　题：aqueous metal-ion batteries aqueous alkali metal-ion batteries zinc-ion batteries interfacial behavior stationary energy storage 

摘      要：Rechargeable aqueous metal-ion batteries(AMBs)have attracted extensive scientific and commercial interest due to their potential for cost-effective,highly safe,and scalable stationary energy ***,their limited output voltage,inadequate energy density,and poor reversibility of ambiguous electrode reactions in aqueous electrolytes strongly limit their practical *** review aims to elucidate the challenges of existing AMBs from the material design to whole device *** summarize the emerging electrochemistry,fundamental properties,and key issues in interfacial behaviors of various classes of prevailing AMBs,including aqueous alkali metal-ion batteries and multivalent-ion batteries,and present an appraisal of recent advances for addressing the performance ***,the progress of zinc-ion batteries is highlighted to provide a ubiquitous guideline for their commercialization in the grid-scale energy ***,we figure out the dominating general challenges for achieving high-performance AMBs,laying out a perspective for future breakthroughs.