Evaluation of solid electrolytes: Development of conventional and interdisciplinary approaches
作者机构：College of PhysicsQingdao UniversityQingdaoChina College of Materials Science and EngineeringQingdao UniversityQingdaoChina
出 版 物：《Interdisciplinary Materials》 (交叉学科材料（英文）)
年 卷 期：2023年第2卷第4期
页 面：529-568页
核心收录：
基 金：supported by the National Natural Science Foundation of China(Grant Nos.U1932205 and 52002197) the Key R&D Program of Shandong Province(Grant No.2021CXGC010401)
主 题：advanced characterization interdisciplinary techniques machine learning solid electrolytes solid-state batteries
摘 要：Solid-state lithium batteries(SSLBs)have received considerable attention due to their advantages in thermal stability,energy density,and *** electrolyte(SE)is a key component in developing high-performance *** in-depth understanding of the intrinsic bulk and interfacial properties is imperative to achieve SEs with competitive *** review first introduces the traditional electrochemical approaches to evaluating the fundamental parameters of SEs,including the ionic and electronic conductivities,activation barrier,electrochemical stability,and diffusion *** that,the characterization techniques to evaluate the structural and chemical stability of SEs are ***,emerging interdisciplinary visualization techniques for SEs and interfaces are highlighted,including synchrotron X-ray tomography,ultrasonic scanning imaging,time-of-flight secondary-ion mass spectrometry,and three-dimensional stress mapping,which improve the understanding of electrochemical performance and failure *** addition,the application of machine learning to accelerate the screening and development of novel SEs is *** review article aims to provide an overview of advanced characterization from a broad physical chemistry view,inspiring innovative and interdisciplinary studies in solid-state batteries.
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