Perspective on powder technology for all-solid-state batteries:How to pair sulfide electrolyte with high-voltage cathode

作     者：Jiangkui Hu Shijie Yang Yingying Pei Xilong Wang Yulong Liao Shuai Li Aolong Yue Jia-Qi Huang Hong Yuan Jiangkui Hu;Shijie Yang;Yingying Pei;Xilong Wang;Yulong Liao;Shuai Li;Aolong Yue;Jia-Qi Huang;Hong Yuan

作者机构：School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing100081China Advanced Research Institute of Multidisciplinary ScienceBeijing Institute of TechnologyBeijing100081China 

出 版 物：《Particuology》 (颗粒学报（英文版）)

年 卷 期：2024年第86卷第3期

页      面：55-66页

核心收录：

学科分类：0808[工学-电气工程] 0817[工学-化学工程与技术] 08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：supported by the Beijing Natural Science Foundation(grant No.L223009) the National Natural Science Foundation of China(grant No.22075029) the National Key Research and Development Program of China(grant No.2021YFB2500300) the Key Research and Development(R&D)Projects of Shanxi Province(grant No.2021020660301013) 

主　　题：Sulfide solid electrolytes High-voltage cathodes Electrode/electrolyte interfaces All-solid-state lithium batteries 

摘      要：Sulfide solid electrolytes(SEs)have attracted ever-increasing attention due to their superior roomtemperature ionic conductivity(~10^(-2) S cm^(-1)).Additionally,the integration of sulfide SEs and highvoltage cathodes is promising to achieve higher energy ***,the incompatible interfaces between sulfide SEs and high-voltage cathodes have been one of the key factors limiting their ***,this review presents a critical summarization of the interfacial issues in all-solid-state lithium batteries based on sulfide SEs and high-voltage cathodes and proposes strategies to stabilize the electrolyte/cathode ***,the future research direction of electrolyte/cathode interfaces and application prospects of powder technology in sulfide-based ASSLBs were also discussed.