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Construction of oxygen-vacancies-rich S-scheme BaTiO_(3)/red phosphorous heterojunction for enhanced photocatalytic activity

作     者:Yuhua Ma Xiadiye Aihemaiti Kezhen Qi Shiyin Wang Yanjie Shi Zhuanhu Wang Minghe Gao Fuhe Gai Yulian Qiu Yuhua Ma;Xiadiye Aihemaiti;Kezhen Qi;Shiyin Wang;Yanjie Shi;Zhuanhu Wang;Minghe Gao;Fuhe Gai;Yulian Qiu

作者机构:College of Chemistry and Chemical EngineeringXinjiang Normal UniversityUrumqi 830054China Xinjiang Key Laboratory of Energy Storage and Photoelectrocatalytic MaterialsXinjiang Normal UniversityUrumqi 830054China College of PharmacyDali UniversityDali 671000China 

出 版 物:《Journal of Materials Science & Technology》 (材料科学技术(英文版))

年 卷 期:2023年第156卷第25期

页      面:217-229页

核心收录:

学科分类:0830[工学-环境科学与工程(可授工学、理学、农学学位)] 081704[工学-应用化学] 081705[工学-工业催化] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070304[理学-物理化学(含∶化学物理)] 0703[理学-化学] 

基  金:financially supported by the National Natu-ral Science Foundation of China(Nos.52063028,22208275 and 22268003) the Ph.D.Startup Fund of Xinjiang Normal Univer-sity(No.XJNUBS1907) the Xinjiang Normal University Outstanding Young Teachers’Research Initiation Project(No.XJNU202015) the Innovation team for monitoring of emerging contaminants and biomarkers(No.2021D14017) 

主  题:S-scheme heterojunction Red phosphorous BaTiO3 Photocatalytic activity 

摘      要:The S-scheme heterojunctions can effectively separate photogenerated electrons and holes,retain their high redox capacity,and provide great prospects for enhancing the photocatalytic activity of the composites in different ***,S-scheme heterojunction photocatalytic materials were rationally designed and prepared by a simple hydrothermal method between narrow-bandgap red phosphorus(HRP)and wide-bandgap BaTiO_(3)(BTO)*** to the effective charge separation and redox ability from the S-scheme mechanism and oxygen vacancies,BTO/HRP exhibited good photoelectrochemical and photocatalytic degradation *** photoreaction tests demonstrated that BTO/HRP had high practicality in the removal of pollutants from wastewater;its photodegradation rate of Rhodamine B reached 3.029×10^(−1) min^(−1) in 12 min;and it could inactivate 1.8×10^(9) CFU/mL of *** in 1 h,with an antibacterial rate of 99.8%.This paper provided a promising photocatalyst for pollutant removal and a new strategy for the fabrication of efficient RP-based photocatalytic materials.

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