Modulation of morphology and electronic structure on MoS_(2)-based electrocatalysts for water splitting
作者机构：College of Science&School of Plant ProtectionAnhui Agricultural UniversityHefei 230036China Shenyang National Laboratory for Materials ScienceInstitute of Metal ResearchChinese Academy of SciencesShenyang 110016China
出 版 物：《Nano Research》 (纳米研究（英文版）)
年 卷 期：2022年第15卷第8期
页 面：6862-6887页
核心收录：
学科分类：07[理学] 070304[理学-物理化学(含∶化学物理)] 0805[工学-材料科学与工程（可授工学、理学学位）] 0703[理学-化学] 0702[理学-物理学]
基 金：the National Natural Science Foundation of China(No.21902157) Starting fund for scientific research of high-level talents,Anhui Agricultural University(No.rc382108) the Open Fund of The State Key Laboratory of Catalysis in DICP,CAS(N-21-12) the Open Fund of The State Key Laboratory of Molecular Reaction Dynamics in DICP,CAS(SKLMRDK202223).
主 题：MoS_(2) morphology electronic structure electrocatalysis water splitting
摘 要：Electrocatalytic water splitting into hydrogen is one of the most favorable approaches to produce renewable energy.MoS_(2)has received great research attention for both hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)due to its unique structure and ability to be chemically modified,enabling its electrocatalytic activity to be further enhanced or made comparable to that of Pt-based materials.In this review,we discuss the important fabrication approaches of MoS_(2)ultrathin nanosheet(MoS_(2)NS)to improve the intrinsic catalytic activity of bulk MoS_(2).Moreover,several modification strategies involve either morphology modulation or electron structural modulation to improve the charge transfer kinetics,including doping,vacancy,and heterojunction construction or single-atom anchor.Our perspectives on the key challenges and future directions of developing high-performance MoS_(2)-based electrocatalysts for overall water splitting are also discussed.
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