Defect engineering of electrocatalysts for organic synthesis
作者机构：Key Laboratory of Chemo/Bio-Sensing and ChemometricsCollege of Chemistry and Chemical EngineeringAdvanced Catalytic Engineering Research Center of the Ministry of EducationHunan UniversityChangsha 410082China School of Chemistry and Chemical EngineeringJishou UniversityJishou 416000China
出 版 物：《Nano Research》 (纳米研究（英文版）)
年 卷 期：2023年第16卷第2期
页 面：1890-1912页
核心收录：
学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070303[理学-有机化学] 0703[理学-化学]
基 金：supported by the National Key Research and Development Program of China(No.2020YFA0710000) the National Natural Science Foundation of China(Nos.22122901 and 21902047) the Provincial Natural Science Foundation of Hunan(Nos.2020JJ5045,2021JJ20024,and 2021RC3054) the Shenzhen Science and Technology Program(No.JCYJ20210324140610028)
主 题：defect engineering electrocatalysts electrocatalytic organic synthesis energy conversion
摘 要：Electrocatalytic organic synthesis has attracted considerable research attention because it is an efficient and eco-friendly strategy for converting energy sources to value-added *** engineering is a promising strategy for regulating the electronic structure and charge density of *** endows electrocatalysts with excellent physical and physicochemical properties and optimizes the adsorption energy of the reaction intermediates to reduce the kinetic barriers of the electrosynthesis ***,the recent advances related to the use of electrocatalysts for organic synthesis with respect to defects are systematically *** roles of defects in anodic and cathodic reactions,such as the syntheses of alkanes,alkenes,alcohols,aldehydes,amides,and carboxylic acids,are ***,the relationship between the defective structure and electrocatalytic activity is discussed by combining experimental results and theoretical ***,the challenges,opportunities,and development prospects of defective electrocatalysts are examined to promote the development of the field of electrocatalytic organic *** review is expected to help understand the vital role of defects in catalytic processes and the controllable synthesis of efficient electrocatalysts for the production of high-value chemicals.
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