Two-Dimensional Cathode Materials for Aqueous Rechargeable Zinc-Ion Batteries

作     者：Yurou Wang Jun Yin Jian Zhu Yurou Wang;Jun Yin;Jian Zhu

作者机构：School of Materials Science and EngineeringNankai UniversityTianjin 300350China 

出 版 物：《Chinese Journal of Chemistry》 (中国化学（英文版）)

年 卷 期：2022年第40卷第8期

页      面：973-988页

核心收录：

学科分类：0808[工学-电气工程] 08[工学] 0703[理学-化学] 

基　　金：supported by NSFC(Nos.51873088,12004195) Tianjin Municipal Science and Technology Commission(Nos.20JCQNJC01820,18ZLZXZF00480) 111Project(No.B18030)in China. 

主　　题：Two-dimensional materials Zinc-ion batteries Electrochemistry Nanostructures Energy conversion 

摘      要：Rechargeable aqueous zinc-ion batteries(ZIBs)featuring low cost,superior performance,and environmental benignity have attracted dramatic atten-tion as a promising alternative energy storage system to lithium-ion batteries.Nevertheless,the development of ZIBs is still hindered by the limited selection of cathode materials due to the large solvation sheath and charge density of Zn^(2+).Two-dimensional(2D)materials have attracted extraor-dinary attention owing to the unique layered structure bonded by weak van der Waals forces,which makes them promising host materials for Zn^(2+)intercalation/de-intercalation.In this review,the synthesis and properties of 2D materials for cathodes in ZIBs are discussed.Meanwhile,various re-ports on 2D materials as ZIBs cathodes are summarized.Three key strategies to elicit improved Zn2+storage abilities:defect engineering,hetero-structure engineering,and interlayer engineering,are highlighted.Finally,this review ends with perspectives relating to the challenges and opportu-nities of 2D materials-based ZIBs.