Two-dimensional nanomaterials confined single atoms: New opportunities for environmental remediation

作     者：Yu Yin Lei Shi Shu Zhang Xiaoguang Duan Jinqiang Zhang Hongqi Sun Shaobin Wang Yu Yin;Lei Shi;Shu Zhang;Xiaoguang Duan;Jinqiang Zhang;Hongqi Sun;Shaobin Wang

作者机构：School of Environmental and Chemical EngineeringJiangsu University of Science and TechnologyZhenjiang212100China Joint International Research Laboratory of Biomass Energy and MaterialsCollege of Materials Science and EngineeringNanjing Forestry UniversityNanjing210037China School of Chemical Engineering and Advanced MaterialsThe University of AdelaideAdelaideSA5005Australia School of ScienceEdith Cowan UniversityJoondalupWA6027Australia 

出 版 物：《Nano Materials Science》 (纳米材料科学（英文版）)

年 卷 期：2023年第5卷第1期

页      面：15-38页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 07[理学] 070205[理学-凝聚态物理] 08[工学] 080501[工学-材料物理与化学] 0805[工学-材料科学与工程（可授工学、理学学位）] 0702[理学-物理学] 

基　　金：This work was financially supported by the National Natural Science Foundation of China(51602133,51876093) China MOST(2018YFE0183600) 

主　　题：Single-atom catalysis Two-dimensional material Advanced oxidation process Degradation Transformation Industrial wastewater 

摘      要：Two-dimensional(2D)supports confined single-atom catalysts(2D SACs)with unique geometric and electronic structures have been attractive candidates in different catalytic applications,such as energy conversion and storage,value-added chemical synthesis and environmental ***,their environmental appli-cations lack of a comprehensive summary and in-depth *** this review,recent progresses in synthesis routes and advanced characterization techniques for 2D SACs are introduced,and a comprehensive discussion on their applications in environmental remediation is ***,2D SACs can be effective in catalytic elimination of aqueous and gaseous pollutants via radical or non-radical routes and transformation of toxic pollutants into less poisonous species or highly value-added products,opening a new horizon for the contami-nant *** addition,in-depth reaction mechanisms and potential pathways are systematically discussed,and the relationship between the structure-performance is ***,several critical challenges within this field are presented,and possible directions for further explorations of 2D SACs in environmental remediation are *** the research of 2D SACs in the environmental application is still in its infancy,this review will provide a timely summary on the emerging field,and would stimulate tremendous interest for designing more attractive 2D SACs and promoting their wide applications.