Recent progress on two-dimensional materials confining single atoms for CO_(2) photoreduction

作     者：Xianjin Shi Leo NYCao Meijuan Chen Yu Huang Xianjin Shi;Leo N.Y.Cao;Meijuan Chen;Yu Huang

作者机构：Key Laboratory of Aerosol Chemistry and PhysicsState Key Laboratory of Loess and Quaternary Geology(SKLLQG)Institute of Earth EnvironmentChinese Academy of SciencesXi'an 710061China Center of Excellence in Quaternary Science and Global ChangeChinese Academy of SciencesXi'an 710061China University of Chinese Academy of SciencesBeijing 100049China CAS Center for Excellence in NanoscienceBeijing Key Laboratory of Micro-nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 101400China School of Nanoscience and TechnologyUniversity of Chinese Academy of SciencesBeijing 100049China School of Human Settlements and Civil EngineeringXi'an Jiaotong UniversityXi'an 710049China 

出 版 物：《Chinese Chemical Letters》 (中国化学快报（英文版）)

年 卷 期：2022年第33卷第12期

页      面：5023-5029页

核心收录：

学科分类：081704[工学-应用化学] 081705[工学-工业催化] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 080501[工学-材料物理与化学] 0805[工学-材料科学与工程（可授工学、理学学位）] 0703[理学-化学] 

基　　金：supported by the Strategic Priority Research Program of the Chinese Academy of Sciences,China(Nos.XDA23010300 and XDA23010000) National Science Foundation of China,China(Nos.51878644 and 41573138) the National Key Research and Development Program of China,China(No.2016YFA0203000) the Plan for"National Youth Talents"of the Organization Department of the Central Committee 

主　　题：CO_(2)reduction Photocatalyst Single atom 2D materials g-C_(3)N_(4) 

摘      要：Photoreduction of CO_(2) into value-added products offers a promising approach to overcome both climate change and energy ***,low conversion efficiency,poor product selectivity,and unclear mechanism limit the further advancement of CO_(2) *** development of two-dimensional(2D)materials and construction of single atom sites are two frontier research fields in *** the advantages of 2D materials and single atom sites is expected to make a breakthrough in CO_(2) *** this review,we summarized the design and application,proposed challenges and opportunities,and laid a foundation for further research and application of 2D materials confining single atoms(SACs@2D)for CO_(2) photoreduction.