Advanced inorganic/polymer hybrid electrolytes for all-solid-state lithium batteries
作者机构：Science and Technology on Advanced Ceramic Fibers and Composites LaboratoryCollege of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China South China Advanced Institute for Soft Matter Science and TechnologySchool of Molecular Science and EngineeringSouth China University of TechnologyGuangzhou 510640China Department of Chemical and Environmental EngineeringYale UniversityNew Haven 06511USA
出 版 物：《Journal of Advanced Ceramics》 (先进陶瓷（英文）)
年 卷 期：2022年第11卷第6期
页 面：835-861页
核心收录：
基 金：This work was financially supported by the National Natural Science Foundation of China(No.22003017) the National Key R&D Program of China(No.2018YFB1900603) Natural Science Foundation of Guangdong Province(No.2020A1515011506) Xiaoyu JI is thankful for the financial support from the China Scholarship Council(No.201903170199)for his visit to Yale University The authors thank Prof.Mingjiang ZHONG(Yale University)and Prof.Stephen Z.D.CHENG(University of Akron)for their helpful discussion
主 题：solid-state electrolytes(SSEs) hybrid electrolytes energy density electrical energy storage(EES) lithium batteries
摘 要：Solid-state batteries have become a frontrunner in humankind’s pursuit of safe and stable energy storage systems with high energy and power *** materials,currently,seem to be the Achilles’heel of solid-state batteries due to the slow kinetics and poor interfacial *** the merits of solid inorganic electrolytes(SIEs)and solid polymer electrolytes(SPEs),inorganic/polymer hybrid electrolytes(IPHEs)integrate improved ionic conductivity,great interfacial compatibility,wide electrochemical stability window,and high mechanical toughness and flexibility in one material,having become a sought-after pathway to high-performance all-solid-state lithium ***,we present a comprehensive overview of recent progress in IPHEs,including the awareness of ion migration fundamentals,advanced architectural design for better electrochemical performance,and a perspective on unconquered challenges and potential research *** review is expected to provide a guidance for designing IPHEs for next-generation lithium batteries,with special emphasis on developing high-voltage-tolerance polymer electrolytes to enable higher energy density and three-dimensional(3D)continuous ion transport highways to achieve faster charging and discharging.
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