One-step Synthesis and Photocatalytic Degradation Performance of Sulfur-doped Porous g-C_(3)N_(4)Nanosheets
One-step Synthesis and Photocatalytic Degradation Performance of Sulfur-doped Porous g-C3N4 Nanosheets作者机构:School of Petrochemical EngineeringLiaoning Petrochemical UniversityLiaoning 113001
出 版 物:《China Petroleum Processing & Petrochemical Technology》 (中国炼油与石油化工(英文版))
年 卷 期:2022年第24卷第1期
页 面:81-89页
核心收录:
学科分类:0820[工学-石油与天然气工程] 07[理学] 081705[工学-工业催化] 070205[理学-凝聚态物理] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0703[理学-化学] 0702[理学-物理学]
基 金:supported by the Liaoning Provincial Natural Fund Mentoring Program Project (2019-ZD-0057)
主 题:sulfur-doped g-C3N4 nanosheets photocatalysis degradation
摘 要:In this study,the sulfur-doped porous g-C_(3)N_(4) nanosheets(CN-T-U 1.75)were synthesized successfully by onestep calcination utilizing urea and thiourea as precursors.Under visible light irradiation,CN-T-U 1.75 showed remarkable photocatalytic activity for Rhodamine B(RhB)degradation with a kinetic reaction rate constant of 0.01838 min^(-1).The characterization analysis indicated that CN-T-U 1.75 had a higher specific surface area and the doping altered the energy band structure.This work offers a new viewpoint on modifying the band structure of a photocatalyst using a doping strategy,as well as new insights into the generation routes of active species involved in the photocatalytic process.