CO_(2) reduction with coin catalyst
作者机构：Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsFudan UniversityShanghai 200433China School of Microelectronics and State Key Laboratory of ASIC and SystemFudan UniversityShanghai 200433China
出 版 物：《Nano Research》 (纳米研究（英文版）)
年 卷 期：2022年第15卷第5期
页 面：3859-3865页
核心收录：
学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070303[理学-有机化学] 0703[理学-化学]
基 金：The authors are grateful to the financial support from the National Natural Science Foundation of China(Nos.21771040 and 62074043) the National Key Research and Development Program of China(Nos.2017YFA0207303 and 2016YFA0203900)
主 题：closed-loop lifecycle electrocatalysis coin catalyst
摘 要：Most organic commodity chemicals are derived from fossil carbon *** dependency is so immense that it is difficult to compensate for the accompanying carbon footprint with current technology and chemical *** mitigate the future fossil fuel usage,it is crucial to explore alternative chemical pathways,which are both sustainable and suitable for large-scale *** we demonstrate a closed-loop carbon-neutral chemical route,using standard coin catalyst,to produce high concentrated formate and formic *** catalyst s Faradaic efficiency(FE)of formate is~95.3% with great *** chemicals are not only synthesized but also purified and utilized in zero-carbon *** successfully harvested 45%formate salt and 86.2% formic acid,for applications like anti-freezing reagent and green liquid fuel to power the fuel-cell vehicles.
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