Research progress of defect-engineered UiO-66(Zr)MOFs for photocatalytic hydrogen production
作者机构:School of Chemical Engineering and Material ScienceTianjin University of Science and TechnologyTianjin 300457China School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China
出 版 物:《Frontiers in Energy》 (能源前沿(英文版))
年 卷 期:2021年第15卷第3期
页 面:656-666页
核心收录:
学科分类:0808[工学-电气工程] 07[理学] 070304[理学-物理化学(含∶化学物理)] 0807[工学-动力工程及工程热物理] 0703[理学-化学]
基 金:This work was supported by the Scientific Research Project of Tianjin Municipal Education Commission(Grant No.2019KJ221) the Chemistry and Chemical Engineering Guangdong Laboratory(Grant No.1912011).
主 题:defect engineering metal-organic frameworks UiO-66 photocatalysis
摘 要:In recent years,defect-engineered Zr-based UiO-66 metal-organic frameworks(UiO-66(Zr)metalorganic frameworks(MOFs))have shown huge advantages in catalytic,functional materials,adsorption,and other fields due to their large surface areas,well-ordered porous structures,and flexible tailorability.It is extremely challenging to introduce defect sites in the synthesis of MOFs to regulate the physicochemical properties of materials such as(energy band structure,pore structure,etc.)to obtain an excellent performance.This paper reviews the recent research results of synthesis methods,characterization technologies,and application fields of defect-engineered UiO-66(Zr)MOFs materials in order to provide new insights to synthesize high-performance UiO-66(Zr)MOFs materials and promote the development of UiO-66(Zr)in various fields.