Roles of Metal-Free Materials in Photoelectrodes for Water Splitting

作     者：Xiaochun Li Jiawen Wang Yuanxing Fang Hong Zhang Xianzhi Fu Xinchen Wang 

作者机构：State Key Laboratory of Photocatalysis on Energy and EnvironmentCollege of ChemistryFuzhou UniversityFuzhou 350116P.R.China 

出 版 物：《Accounts of Materials Research》 (材料研究述评（英文）)

年 卷 期：2021年第2卷第10期

页      面：933-943页

学科分类：081704[工学-应用化学] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0805[工学-材料科学与工程（可授工学、理学学位）] 0703[理学-化学] 

基　　金：This work was supported by the National Natural Science Foundation of China(21961142019,22075047,U1905214,and 21861130353) the National Key R&D Program of China(2018YFA0209301) the 111 Project(D16008) the Chang Jiang Scholars Program of China(T2016147) 

主　　题：stability. kinetics breakthrough 

摘      要：CONSPECTUS:Photoelectrochemical(PEC)water splitting is an appealing approach to the hydrogen evolution reaction since it converts sunlight in the form of hydrogen fuel,which has the potential to revolutionize the fossil fuel-based energy systems of the modern *** the last half century,progress has been made with respect to the material,synthesis,and *** developments of multilayered photoelectrodes have made a breakthrough to improve the sunlight conversion efficiency and strengthen the physiochemical *** exploration of new materials for the functional layers of photoelectrodes offers a new opportunity for practical *** the emerging materials,metal-free species have shown superior properties,such as high stability,sustainability,and *** respect to inorganic materials,their physiochemical properties can be readily regulated,including thermodynamics and kinetics,and thus increasing attention has been devoted.