Editing the Shape Morphing of Monocomponent Natural Polysaccharide Hydrogel Films
作者机构：Institute of Biomedical&Health EngineeringShenzhen Institute of Advanced Technology(SIAT)Chinese Academy of Sciences(CAS)Shenzhen 518035China Key Laboratory of Polymeric Materials and Application Technology of Hunan ProvinceKey Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of EducationSchool of ChemistryXiangtan UniversityXiangtan 411105China Institute of Advanced Materials Science and EngineeringShenzhen Institute of Advanced Technology(SIAT)Chinese Academy of Sciences(CAS)Shenzhen 518035China State Key Laboratory of Fluid Power&Mechatronic SystemKey Laboratory of Soft Machines and Smart Devices of Zhejiang ProvinceDepartment of Engineering MechanicsZhejiang UniversityHangzhou 310027China
出 版 物：《Research》 (研究（英文）)
年 卷 期：2021年第2021卷第1期
页 面：835-846页
核心收录：
学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070305[理学-高分子化学与物理] 080501[工学-材料物理与化学] 0805[工学-材料科学与工程（可授工学、理学学位）] 0703[理学-化学]
基 金：supported by the National Key R&D Program of China(2017YFA0701303,2017YFC0111202) the National Natural Science Foundation of China(52022102,52003287) the Youth Innovation Promotion Association of CAS(2019353) the CAS Key Laboratory of Health Informatics,Shenzhen Institutes of Advanced Technology,Chinese Academy of Sciences(2011DP173015) the Foundation of Hunan Educational Committee(18K030) the Shenzhen Science and Technology Innovation Committee(JCYJ20180507182051636,KQJSCX20180330170232019)
摘 要：Shape-morphing hydrogels can be widely used to develop artificial muscles,reconfigurable biodevices,and soft ***,conventional approaches for developing shape-morphing hydrogels highly rely on composite materials or complex manufacturing techniques,which limit their practical ***,we develop an unprecedented strategy to edit the shape morphing of monocomponent natural polysaccharide hydrogel films via integrating gradient cross-linking density and geometry *** to the synergistic effect,the shape morphing of chitosan(CS)hydrogel films with gradient cross-linking density can be facilely edited by changing their geometries(length-to-width ratios or thicknesses).Therefore,helix,short-side rolling,and longside rolling can be easily ***,various complex artificial 3D deformations such as artificial claw,horn,and flower can also be obtained by combining various flat CS hydrogel films with different geometries into one system,which can further demonstrate various shape transformations as triggered by *** work offers a simple strategy to construct a monocomponent hydrogel with geometry-directing programmable deformations,which provides universal insights into the design of shape-morphing polymers and will promote their applications in biodevices and soft robotics.
维普期刊数据库