Enhanced CO_(2)electroreduction to ethylene via strong metal-support interaction

作     者：Mengen Chu Chunjun Chen Yahui Wu Xupeng Yan Shuaiqiang Jia Ruting Feng Haihong Wu Mingyuan He Buxing Han Mengen Chu;Chunjun Chen;Yahui Wu;Xupeng Yan;Shuaiqiang Jia;Ruting Feng;Haihong Wu;Mingyuan He;Buxing Han

作者机构：Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesSchool of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai200062China Beijing National Laboratory for Molecular SciencesCAS Key Laboratory of Colloid and Interface and ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing100190China 

出 版 物：《Green Energy & Environment》 (绿色能源与环境（英文版）)

年 卷 期：2022年第7卷第4期

页      面：792-798页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 081702[工学-化学工艺] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 

基　　金：supported by the National Key Research and Development Program of China(2017YFA0403102) National Natural Science Foundation of China(21573073,21733011) Beijing Municipal Science&Technology Commission(Z191100007219009) the Chinese Academy of Sciences(QYZDY-SSW-SLH013) 

主　　题：Carbon dioxide reduction Ethyene Electrocatalyst Copper-ceria interaction 

摘      要：The CuO/CeO_(2) composites with strong metal-support interaction were synthesised,which can efficiently electroreduct CO_(2)to C(2)H_(4).The Faradaic efficiency(FE)of C_(2)H_(4) could reach 50.5%with a current density of 18 mA cm^(-2).The strong metal-support interaction could not only enhance the adsorption and activation of CO_(2),but also can stablize the CuO.