Two-Dimensional Electronic Spectroscopy with Active Phase Management

作     者：Wei-da Zhu Rui Wang Xiao-yong Wang Min Xiao Chun-feng Zhang 朱伟达;王睿;王晓勇;肖敏;张春峰

作者机构：National Laboratory of Solid State MicrostructuresSchool of Physicsand Collaborative Innovation Center for Advanced MicrostructuresNanjing UniversityNanjing 210093China Department of PhysicsUniversity of ArkansasFayettevilleArkansas 72701United States of America 

出 版 物：《Chinese Journal of Chemical Physics》 (化学物理学报（英文）)

年 卷 期：2021年第34卷第1期

页      面：30-42,I0011页

核心收录：

学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070302[理学-分析化学] 0703[理学-化学] 0702[理学-物理学] 

基　　金：This work is supported by the National Key R&D Program of China(No.2017YFA0303700 and No.2018YFA0209101) the National Natural Science Foundation of China(No.21922302,No.21873047,No.11904168,No.91833305,and No.91850105) the Priority Academic Program Development of Jiangsu Higher Education Institutions the Fundamental Research Funds for the Central University 

主　　题：Two-dimensional electronic spectroscopy Active phase management Frequency comb 

摘      要：Two-dimensional elec tronic spec troscopy(2DES)is a powerful met hod to probe the coherent electron dynamics in complicated *** the phase difference of the incident ultrashort pulses is the mos t challenging par t for experimen tal demonstration of ***,we present a tuto rial review on the 2DES proto cols based on active phase managements which are originally developed for quantum optics *** introduce the 2DES techniques in box and pump-probe geometries with phase stabilization realized by interferometry,and outline the fully collinear 2DES approach with the frequency tagging by acoustic optical modulators and frequency *** combination of active phase managements,ultrashort pulses and other spectroscopic methods may open new opportunities to tackle essential challenges related to excited states.