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Scalable salt-templated directed synthesis of high-quality MoS_(2) nanosheets powders towards energetic and environmental applications

作     者:Lijie Zhu Pengfei Yang Yahuan Huan Shuangyuan Pan Zhaoqian Zhang Fangfang Cui Yuping Shi Shaolong Jiang Chunyu Xie Min Hong Jiatian Fu Jingyi Hu Yanfeng Zhang Lijie Zhu;Pengfei Yang;Yahuan Huan;Shuangyuan Pan;Zhaoqian Zhang;Fangfang Cui;Yuping Shi;Shaolong Jiang;Chunyu Xie;Min Hong;Jiatian Fu;Jingyi Hu;Yanfeng Zhang

作者机构:Department of Materials Science and EngineeringCollege of EngineeringPeking UniversityBeijing100871China 

出 版 物:《Nano Research》 (纳米研究(英文版))

年 卷 期:2020年第13卷第11期

页      面:3098-3104页

核心收录:

学科分类:0808[工学-电气工程] 07[理学] 0809[工学-电子科学与技术(可授工学、理学学位)] 070205[理学-凝聚态物理] 0805[工学-材料科学与工程(可授工学、理学学位)] 0702[理学-物理学] 

基  金:supported by the National Key Research and Development Program of China(No.2018YFA0703700) the National Natural Science Foundation of China(Nos.51991340,51991344,and 51861135201) the Beijing Natural Science Foundation(No.2192021). 

主  题:mass production salt-templated molybdenum disulfide chemical vapor deposition green transfer 

摘      要:Two-dimensional(2D)transition metal dichalcogenides(TMDCs)have emerged as perfect platforms for developing applications in nano-electronics,catalysis,energy storage and environmental-related fields due to their superior properties.However,the low-cost,batch production of high-quality 2D TMDCs remains a huge challenge with the existing synthetic strategies.Herein,we present a scalable chemical vapor deposition(CVD)approach for the batch production of high-quality MoS_(2) nanosheet powders,by using naturally abundant,water-soluble and recyclable NaCl crystal powders as templates.The high-quality MoS_(2) nanosheets powders are achieved by a facile water dissolution-filtration process,by virtue of the excellent dispersibility of the as-grown products in water.The internal mechanism for the scalable synthesis strategy is explored.The applications of the MoS_(2) nanosheets powders are also demonstrated as catalysts or adsorbents in hydrogen evolution reaction(HER)and organic dyes adsorption,respectively.This work should hereby pave ways for the mass production and application of powdery TMDCs in energetic and environmental related fields.

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