A review of pulse electrolysis for efficient energy conversion and chemical production
A review of pulse electrolysis for efficient energy conversion and chemical production作者机构：Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsFudan University200438 ShanghaiChina National Engineering Laboratory for Industrial Wastewater TreatmentEast China University of Science and Technology200237 ShanghaiChina
出 版 物：《Journal of Energy Chemistry》 (能源化学（英文版）)
年 卷 期：2021年第30卷第8期
页 面：69-82,I0003页
核心收录：
学科分类：081704[工学-应用化学] 08[工学] 0817[工学-化学工程与技术]
基 金：supports from the National Key R&D program of China(2019YFC1604602) supports from the National Key Basic Research Program of China(2019YFC1906700) the National Natural Science Foundation of China(21876049,51878643)
主 题：Pulse electrolysis Energy conversion Chemical production Water splitting CO_(2) reduction Energy electrocatalysis
摘 要：Electrochemical transformation emerges as an important solution to sustainable energy conversion and chemical *** electrolytic systems usually operate under galvanostatic or potentiostatic conditions that sometimes result in unsatisfactory efficiencies or *** electrolysis by pulsating and programming the potentials/currents can feature unique tunability to the electrodeelectrolyte interface properties that can give rise to drastically different electrochemical behaviors compared to the steady-state *** invented almost 100 years ago,pulse electrolysis has received little attention over the period,but has recently attracted a revived focus toward the energyefficient *** review will summarize the history and recent efforts of pulse electrolysis in three categories:water electrolysis,CO_(2)electrolysis and other *** each section,the advantage of pulse electrolysis over steady-state electrolysis will be discussed in detail,giving a comprehensive overview of the pulse effect on the electrolytic ***,we will provide our vision of future directions in pulse electrolysis based on previous works.
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